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1.3 Risk Factors for Radiation Exposure

Exposure Levels at which Health Effects Appear in Healthy Adults _____________________________________________________

Effects Acute dose (Gy)

_____________________________________________________

Blood count changes 0.50 Vomiting (threshold) 1.00 Mortality (threshold) 1.50 LD50/60 (minimal supportive care) 3.2-3.6 LD50/60 (supportive medical treatment) 4.8-5.4 LD50/60 (autologous bone marrow or stem cell transplant) >5.4

_____________________________________________________

Source: NCRP Report 98 "Guidance on Radiation Received in Space Activities", NCRP, Bethesda(MD) (1989).

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Biological Effects of Radiation

(3)

Energy Loss of Radiation

As higher the energy of the

radiation, as deeper penetration into the surface of the material!

The energy loss depends on E and charge z of radiation particle.

Bragg-Curve: radiation with

certain energy E reaches a certain range R where most of the

radiation particles are stopped!

R dE

dE dx

m

z f E

E

=

0 2 ( )

dE

dxz2f E( )

(4)

Monte Carlo simulation

of electron scattering

(5)

Depth Profiling with Radiation

Radiation can be used for depth profiling!

charge z and mass m of radiation determines depth resolution ∆R

electrons alphas

R

0.5 1.0

Rel. Intensity

depth

∆Rα

∆Re

Interaction between radiation and matter takes place over depth range of penetration Ö signature

(6)

Origin of Radiation

Natural Radioactivity:

• long-lived radioactivity has originated in Supernova explosions prior to solar system;

• or is being produced by Cosmic Ray bombardment of earth atmosphere.

Man-made Radioactivity:

• Accelerator based experiments

• Reactor based experiments

(7)

Man-Made Radioactivity

(8)

Exposure to Natural and Man-Made Radioactivity

Tobacco contains α-emitter

210Po with T1/2=138.4 days.

Through absorption in

bronchial system smoking adds 280 mrem/year to the annual dose of US population

(9)

Sources of Natural and Radioactivity

(10)

Spectrum of CR

Cosmic Rays origin from:

• solar flares;

• distant supernovae;

Cosmic Ray Bombardment

Low energy CR

High energy CR

(11)

Cosmic Rays in High Altitude

Earth is relatively protected from cosmic rays through atmosphere shield; typical exposure is H=3.2 µrem/h. Mountain climbers and

airline crews and passengers are exposed to higher doses of radiation.

Dose doubles every 1500 m in height. At 10 km height dose is about 100 times sea-level dose H=0.32mrem/h.

Example: Total dose H:

• after 10h of flight:

H=3.2 mrem,

• for round trip:

H=6.4 mrem

• Frequent flyer with about 10 transatlantic flights/year H=64 mrem/year.

Compare to natural dose (100 mrem/y) !

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Drastic Effects!

Wife’s ring with ground level dose!

Husband’s ring with transatlantic high altitude dose

Au γ-activity

Ö 8 times

more dose

(13)

14 C Enrichment in Environment

14C is produced by interaction of cosmic rays with 14N in the

atmosphere. Fall out of 14C and implementation into bio-material by photosynthesis. Decay counting may start after bio-material is dead.

(14)
(15)

Evolution of Carbon Content in our Atmosphere

Steady increase through industrial activities and exhaust causes change In atmospheric carbon

14C content!

(16)

14 C/ 12 C Ratio in Atmosphere

Based on ice-and tree-ring calibrations it was determined that 14C/12C ratio is

not constant with time, correction necessary!

Average ratio:14C/12C=1.3·10-12

(17)

Carbon dating example

(18)

[ ]

[ ]

The piece of carbon has a mass of M 25 g. This translates into the number of carbon 12 atoms:

=

= =

=

C N( C N nuclei mole

A g mole M . [nuclei mole]

g mole g

12 A

6 022 1023

12 25

) [ ]

[ ] 1 mole of material has a mass of A [g]!

e.g. 1 mole 12C ≡ 12 g; 1 mole 56Fe 56 g;

1 mole 197Au 197g; 1 mole of 208Pb 208 g 1 mole AlO3 27 g + 3·16 g = 75 g

You find in the ruins of a lost city - in a cold forgotten fireplace - a 25g piece of

charcoal. How much carbon is in there?

Some Reminder?

1 mole of any kind of material contains NA= 6.022·1023 particles (Avogadro’s number)

N(12C) = 1.25 ·1024 atoms

(19)

14 C-Dating, how old is the piece of charcoal?

[ ] [ ] [ ]

[ ]

λ

λ

λ λ

= =

=

=

= ⋅ ⋅ =

= ⋅ =

= = =

− ⋅

ln .

. .

) . [ ];

) . . . [ ]

) min]

( )

ln ( ) ln

. ;

2 0 693

5730 315 10 384 10

125 10

125 10 13 10 163 10

370

370 250 384 10

1 2 7

12 1

12 24

14 12 14 24 12 12

0

14

0

0

12 1

T y s y s

N( C atoms

C C N( C atoms

A N( C [decays

A t A e t

A A t

s t

t

number of C atoms in wood:

if has been constant

initial activity:

12

= 3250[ ]y

You analyze some weak activity of A(t)=dN/dt=250 decays/min, this gives you the clue for determining its age.

The atmospheric ratio is:

14 12

13 10 12

C

C = .

(20)

Sources of Natural Terrestrial Material

Natural alpha decay chains from long-lived heavy radioisotopes

Uranium Series: 238U Ö 206Pb +8α

• Actinium Series: 235U Ö 207Pb +7α

• Thorium Series: 232Th Ö 208Pb +6α

• Neptunium Series: 241Pu Ö 209Pb +8α

There are several long-lived α-emitters in the chain: 234U

230Th, 226Ra!

(21)

Natural Radioactivity in the US

(22)

Long lived 40 K Radioactivity

40K

40Ar 40Ca

β+ β-

γ

40K has a half-life of T1/2=1.28·109 years its natural abundance is 0.0118 %

Potassium-Argon dating method

40Ar

40K

(23)

Internal γ Glowing

On average, 0.27% of the mass of the human body is potassium K of which 0.021% is radioactive 40K with a half-life of T1/2=1.25·109 [y].

Each decay releases an average of Eavg= 0.5 MeV β- and γ-radiation, which is mostly absorbed by the body

but a small fraction escapes the body.

Calculate, how many radioactive

40K atoms are in your body system!

(24)

Some Mass and Number Considerations

[ ] [ ]

[ ]

[

particles

]

N kg

m N

g particles m

N

N particles

g m m

m

atoms K

g

m .

m .

m

m .

m m

K K body

body K

K body

K body

body K K

body K

body

20 15

7 23

7

23 40

7 40

10 83 . 6 :

body 80

for

gramm.

in mass

body the

need you

, calculate

to

/ 10

54 . 8

40

10 67 . 5 10

023 . 10 6

67 . 5

10 023 . 6 of

40

10 67 5 00021

0 :

body in the

K e

radioactiv of

mass

0027 0

: body in the

K potassium of

mass

: body the

of mass

40 40

40

40 40

40

=

=

=

=

=

=

=

(25)

Example: 40 K

Calculate the absorbed body dose over an average human lifetime of t = 70 y for this source of internal exposure.

[ ]

∗ = = ⋅ ⋅

∗ = ⋅ = ⋅

= ⋅

⋅ ⋅ ⋅ ⋅ ⋅

= ⋅ = ⋅ = ⋅

= ⋅

Dose D E

m t A K E

m

Activity A K N T N

D y g m MeV

m

D MeV kg J kg Gy

with eV J

absorbed body

avg body

K K

body

body

: ( )

: ( ) ln

[ ] ln

( . [ ] ) . [ ]

. . [ / ] . [ ]

: [ ] . [ ]

40

40

1 2

15 1

10 2 2

19

40

2

40

70 2

4 88 10 0 5

9 47 10 15 10 15 10

1 1602 10

λ

1.25 10 [y]

9 8.54

[ ] [ ] [ ]

[ ] eV [ ] J

with

Gy kg

J kg

MeV D

19

2 2

11

10 602

. 1 1

:

10 63

. 2 /

10 63

. 2 /

10 66

. 1

=

=

=

=

(26)

Why do we die?

Lifetime dose from K is:

since and radiation has a weighting factor of the equivalent lifetime dose is:

40

D Gy

Q

H D Sv

= ⋅

− ≈

= ⋅ = ⋅

15 10

1

1 15 10

2

2

. [ ]

. [ ]

β γ

2.6·10

-2

2.6·10

-2

The risk for radiation induced fatal cancer is 5·10-2 [Sv-1], Ö the overall risk for 40K radiation self-induced cancer is 0.13%.

40K-activity is powerful tool in archaeology and anthropology

(27)

Summary

Natural radioactivity provides a unique tool;

• characteristic decay patterns allow to analyze the content of the material

• characteristic decay times allow to introduce

radioactive clocks for dating the material

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