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Classification of Single Particle Optical Scattering Patterns

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Classification of Single Particle Optical Scattering

Patterns

G. F. Crosta

Universit`a degli Studi Milano - Bicocca, Italy

Some experimental methods such as TAOS [1] are capable of collecting the light scattered by single airborne particles in the micrometer size range when the latter are illuminated by a triggered laser source (wavelength = 532 nm). Data consist of intensity patterns (Fig. 1) collected in a suitable solid angle at a high rate (>100 patterns per second).

Figure 1.

Typical scattering pattern (a07b03b) produced by an aerosol particle from skid braking tests on a car racing track. Aerosol was collected by an 8-stage impactor device, re-suspended in water

Figure 2: Classification of TAOS patterns from environmental aerosol particles: train on{1,2}→recognize{4}, 142.88432 < ϕ < 168.517815, 86.083414 < ϑ < 93.948435, Exec = w05, δ = 45deg, p = 2.2, d + 1 = 10, axis = u1, 0 <= |u| <= 255, dim[{PC}] = 10.

and injected into the TAOS apparatus.

There is no known theoretical method capable of dete rmining the particle size, shape and complex refractive in dex from such incomplete data. As a consequence a heu ristic algorithm was developed, which relies on spec-trum enhancement for feature extraction and on principal com ponents (PC ) analysis for classification. Spectrum en hancement of an image includes spatial differentiation, possibly of fractional order, followed by non-linear trans-formations aimed at separating structure from tex ture. PC analysis maps each input pattern into a point in the PC space. The classifier was trained with the aim of max-imizing discrimination between suitable sets of TAOS pat-terns e.g., those labelled 1 and 2 in Fig. 2. New sets of patterns e.g., those from skid braking aerosol particles (la-belled 4), were then submitted to the classifier. The result is also displayed by Fig. 2. From the PCs of a given pat-tern one can estimate how much the shape of the particle deviates from the spherical one.

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