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Antiproton stopping power in hydrogen below 120 keV and the Barkas effect / A. ADAMO; AGNELLO M.; F. BALESTRA;
G. BELLI; G. BENDISCIOLI; A. BERTIN; P. BOCCACCIO; G. C. BONAZZOLA; T. BRESSANI; M. BRUSCHI; M. P.
BUSSA; L. BUSSO; D. CALVO; M. CAPPONI; M. CORRADINI; S. COSTA; S. DE CASTRO; D. D'ISEP; I. V.
FALOMKIN; L. FAVA; A. FELICIELLO; L. FERRERO; V. FILIPPINI; R. GARFAGNINI; U. GASTALDI; P. GIANOTTI; A.
GRASSO; C. GUARALDO; F. IAZZI; A. LANARO; E. LODI RIZZINI; M. LOMBARDI; M. P. MACCIOTTA; A. MAGGIORA;
S. MARCELLO; U. MARCONI; G. V. MARGAGLIOTTI; G. MARON; M. MASALA; A. MASONI; I. MASSA; B. MINETTI;
M. MORANDO; M. MORGANTI; D. PANZIERI; G. PAULI; M. PICCININI; R. PIRAGINO; M. POLI; G. B. PONTECORVO;
G. PUDDU; R. A. RICCI; A. ROTONDI; A. M. ROZHDESTVENSKY; P. SALVINI; L. SANTI; M. G. SAPOZHNIKOV; G.
SARTORI; N. SEMPRINI-CESARI; S. SERCI; F. TOSELLO; V. I. TRETYAK; L. VANNUCCI; G. VEDOVATO; L.
VENTURELLI; A. VITALE; A. ZENONI; A. ZOCCOLI; G. ZOSI. - In: PHYSICAL REVIEW A. - ISSN 1050-2947. - 47:5(1993), pp. 4517-4520. [10.1103/PhysRevA.47.4517]
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Antiproton stopping power in hydrogen below 120 keV and the Barkas effect
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12 November 2021
PHYSICAL REVIEW A VOLUME 47, NUMBER 5 MAY 1993
Antiproton stopping power in hydrogen below 120 keV and the Barkas effect A.
Adamo,' M.
Agnello," F.
Balestra,' G.
Belli," G.
Bendiscioli,'
A. Bertin,P. Boccaccio, G. C.
Bonazzola,' T.
Bressani,' M.
Bruschi,M. P.
Bussa,' L.
Busso,' D.
Calvo,'
M.
Capponi,C.
Cicalo,' M.
Corradini,S.
Costa,' I.
D'Antone,S.
De Castro,F.
D'Isep,'
A.
Donzella,I.
V.Falomkin," L.
Fava,' A.
Feliciello,' L.
Ferrero,'
V.Filippini,' D.
Galli,R.
Garfagnini,' U.
Gastaldi,P.
Gianotti,' A.
Grasso,' C.
Guaraldo, 'F.
Iazzi,A.
Lanaro, 'E.
Lodi Rizzini,M.
Lombardi, V.Lucherini, 'A.
Maggiora,' S.
Marcello,'
U. Marconi,G.
Maron, A.Masoni,' I.
Massa,B.
Minetti,M.
Morando,' P.
Montagna,' F.
Nichitiu," D.
Panzieri,'
G.
Pauli,M.
Piccinini,G.
Piragino,' M.
Poli,'G. B.
Pontecorvo," G.
Puddu,' R. A. Ricci,
'"E.
Rossetto,' A.
Rotondi,' A. M.
Rozhdestvensky," P.
Salvini,' L.
Santi,M. G.
Sapozhnikov,"
N. Semprini Cesari,S.
Serci,' P.
Temnikov," S.
Tessaro," F.
Tosello,'
V.I.
Tretyak,'" G. L.
Usai,' L.
Vannucci, gG.
Vedovato,L.
Venturelli,M.
Villa, A.Vitale,G.
Zavattini, A.Zenoni,' A.
Zoccoli, andG.
Zosi'(OBELIX
Collaboration)Dipartimento di Scienze Fisiche, Universita di Cagliari, Cagliari, Italy and Istituto Nazionale diFisica Nucleare, Sezione di Cagliari, I-09100Cagliari, Italy
Politecnico di Torino, Torino, Italy
and Istituto Nazionale diFisica Nucleare, Sezione di Torino, I-10150Torino, Italy Istituto diFisica, Universita di Torino, Torino, Italy
and Istituto Nazionale diFisica Nucleare, Sezione di Torino, I-1'0125Torino, Italy Dipartimento di Elettronica per l'Automazione, Universita degli Studi diBrescia, and Istituto Nazionale diFisicaNucleare, Sezione di Torino, I-25133Brescia, Italy
Dipartimento di FisicaNucleare eTeorica, Universita diPavia, and Istituto Nazionale di FisicaNucleare, Sezione di Pavia, I-27100Pavia, Italy
Dipartimento diFisica, Universita diBologna,
and Istituto Nazionale diFisica Nucleare, Sezione diBologna, I-40100Bologna, Italy
sLaboratori Nazionali diLegnaro dell'Istituto Nazionale di FisicaNucleare,
I
35020Legnaro (P-adoua), Italy"JointInstitute forNuclear Research, Dubna, SUIOIOOOMoscow, R-ussia Laboratori diFrascati dell Istituto Nazionale di FisicaNucleare, I-00044Frascati, Italy
Dipartimento diFisica, Universita diPadova,
and Istituto Nazionale diFisica Nucleare, Sezione diPadova, I-35100Padova, Italy Istituto diFisica, Universita di Trieste,
and Istituto Nazionale di Fisica Nucleare, Sezione di Trieste, I-34127Trieste, Italy Dipartimento diEnergetica, Universita di Firenze, Firenze, Italy
and Istituto Nazionale di FisicaNucleare, Sezione diBologna, I-40100Bologna, Italy Istituto diFisica, Universita di Udine,
and Istituto Nazionale diFisica Nucleare, Sezione di Trieste, I-33100Udine, Italy (Received 27 July 1992)
The simultaneous measurement ofthe spatial coordinates and times ofPs annihilating at rest in aH2 target at very low density p (p/po &
10,
po being the STPdensity) gives the possibility ofevaluating the behavior ofthe pstopping power in H2at low energies (below 120 keV). Itisdifferent from that ofpro- tons (the Barkas effect). Moreover, it isshown that a rise at low-energy values (~
1keV) isneeded to agree with experimental data.PACS number(s): 34.50.Bw
Following the original work
of
Bohr[1]
the high-energy (projectile velocity
))
e /fi) behaviorof
the stop-ping power is very well described by the Bethe [2]formu- la for a point charge penetrating through matter at non- relativistic speed; it is proportional to the projectile charge squared
(Zt ).
Focusing on protons and antipro- tons (p)as projectiles at low velocity (v=e
hrt) the Bornseries is generally assumed to fail and other methods
of
calculating the consequences
of
collision are required. At very low velocity (v(e
/A) a proton loses energy not only in electronic collisions which lead to excitation and ionization; elastic scattering by the screened nuclei is also important.For
protons, the electronic stopping power has a maximum around the typical electron velocity,i. e.
,47 4517 Q~1993The American Physical Society
4518
BRIEF
REPORTS 47=55
keV for H2. Around and below the maximum, mea- surements are not well reproduced by theoretical esti- mates. The electronic contributionto
the total energy loss in hydrogen is commonly assumed (e.g., in published tabulations [3]) to decrease linearly with the proton ve- locity forenergies below 10keV; see alsoRef. [4].
For
antiprotons, even the qualitative behaviorof
the stopping power is only poorly evaluated [5—9]. For
p 's at very low velocities, the energy loss due to excitation and ionization is expected to be considerably enhanced due to the so-called adiabatic ionization processes (see Refs. [5—7]). For
close collisions the passageof
ap inside the orbital radiusof
a target electron will reduce the efFective nuclear charge seen by the electron which will lead to a releaseof
the electron. This fact was first point- ed out by Fermi and Teller[10],
who specifically con- sidered the ground stateof
a system consistingof
a nega- tive muon and a molecule. The molecular mechanism peculiar to the caseof
hydrogen has been worked out by Wightman[5]. For
antiprotons colliding with atomic hy- drogen, Kimura and Inokuti [6]used a molecular-orbital expansion method to show thatif
the antiproton comes within a distanceR„=0.
64ao (ao is the Bohr radius,0.
053nm) from the proton, then the target is ionized (the same R was found by Fermi and Teller).Furthermore, a difference in the stopping power for positive and negative particles (the Barkas effect)
[11]
hasbeen known fora long time, but lack
of
suitable antiparti- cle beams has prohibited quantitative studies [12—23]of
the effect until recent years [24—26].
With the advent
of LEAR
(low-energy antiproton ring) atCERN,
a high-quality beamof
antiprotons at low en- ergies became available, permitting accurate measure- mentsof
the stopping power for antiprotons down to 200 keV [24—
26]and their ionization[27
—29].
To
study pp annihilations at rest, theOBELIX
colla- boration [30]has realized a very low-density hydrogen target, the ratio between the experimental density p and the STP density po ranging from 10 to10,
and a to-tal
of
some 10 annihilation events has been collected.These data are
of
great interest forthe evaluationof
thep stopping power particularly from the energy region just above the maximum down to some hundredsof
eV.The
LEAR
machine deliversto
our experiment a monochromatic 105-MeV/c gr beam, which passes through some materials (aBe
window closing the beam pipe, a thin scintillator detectorSo,
variable air, and My- lar sheets) before entering the ultrapure (less than 1 ppmof
other gases) hydrogen target, 75 cm long and 30cm in diameter. To maximize the fractionof
ps annihilating at rest in the target it is desirable that the largest numberof
ps enter the target volume with a narrow momentum biteand the appropriate nominal momentum. In the best ar- rangement
=45% of
ps are stopped in the Mylar window at the entranceof
the target and the remaining ones enter the target volume with a momentum spectrum ranging from0
to=43
MeV/c. We measure this value with an empty target ((10
mbar) by timeof
flight. More de- tailsof
the experimental technique are given inRef. [30].
We have used three H2 pressure values
(p, =8. 20+0.
05, p2=4. 10+0.
05 p=2. 10+0.
05 mbar)to
which corre-spond three different
E '"(p
)for the kinetic energyof
ps stopping and annihilating in the Hz gas just before the endof
the target. More important, the energy spread (from the minimum zero energy at the entrance) produces a distributionof
the stopping pointsof
the ps in the (z,t)
plane.Figure 1 shows the distribution
of
the experimental mean annihilation times (t,
)in the target as a functionof
the path length (along the z beam direction) for the three values
of
the pressure. Experimentally,t
for each event is measured by the time at which the charged particles produced in the annihilation hit the scintillator barrel surrounding the target, relative to the starting time to given by the p crossing the beam scintillator counter.The time resolution isbetter than 1 ns. The annihilation times distributions are convolutions between the times
of
moderation(t)
until the ps capture and the cascade times(t„,
)of
the protonium atoms. We plotted the distribu- tionof t,
corresponding to abin in zof
2 cm, the experi- mental spatial resolution being 1 cm. We found that all the distributions obtained in this way, well populated sta- tistically, had a constant width and were fully consistent with Gaussian distributions (see Fig. 2). As discussed in Ref.[30],
this circumstance allowed us to determine the (P-p) atom cascade widths. Furthermore, it indicates that a continuous slowing down picture for the p stop- ping power,S(E),
may well be adopted. The error on the experimental mean valuesof t,
foreach bin inzisnegligi- ble.The experimental information contained in Fig. 1may well be related to
S of p.
In fact the p total path length R isevaluated by integrationof S,
700—
rIi 600—
500—
400—
300—
200—
100—
0—
I s i i i I»
i s I«»
I»»
I» «
I«
i g I i i»
I i i i i I0 10 20 30 40 50 60 70 80
Path length (cm)
FICx.1. Bidimensional distributions ofthe mean pp annihila- tion times
(t,
) in the target as a function ofthe annihilation coordinate z for 8.2 mbar, curve a, 4.2 mbar, curve b, and 2.1mbar, curve cH2 pressure values compared with the results of our best-fitting function; seeFig.3.
47
BRIEF
REPORTS 451960
lf} ~p
Q XQ
20
;0
0ZCO 00
I
600 700
Time
(ns)
~Pl m ~~ ~
800 900 1000
FICx.2. Atypical experimental annihilation time distribution for a 2-cm-wide bin for events in the target at aH2 pressure of 2.1mbar.
E
l
EO
I
C3
L
CL0
C 2
CL O (f)
E
dE
=f. -' „,
and, analogously, the mean moderation time tby
10 10
Energy (kev)
10 10
E
dE
t=t t
(2)E;
being the variable kinetic energyof
eachp
at the be- ginningof
the target.Two parameters enter in the annihilation distributions in the target, apart from
S:
(i)the mean kinetic energyof
ps captured by protons (Eca~) and (ii) the mean cascadetime
of
the (p-p) atom,(t,
t), whic—h is different at the three pressures; seeRef. [30].
The experimental data are the(R;, t;+t„,
) mean values for the three situations;0&E; ~E '"(p
) withE '"(p3)(E '"(pz)&E
'"(p&).We outline that, contrary towhat was done with different probes (e.g.,
p
),S
is detertnined, with our technique, by the simultaneous solutionof
both space and time relation- ships (1)and (2). This is possible only with ps, due to their specific featureof
the annihilation and with a so- phisticated and complete apparatus likeOBELIX.
In particular, the useof
(2)allows usto
avoid ambiguities or corrections inevitable in measurements in which only the spatial coordinate relationship (1)is used, and thenS
is derived from the projected range and not from the total range. Moreover, evenif
we suppose that around10% of
events (typically with the higher annihilations times in any 2-cm-wide bin) are characterized by a greater total path length and the proper positioning would be in the neighboring bin, our distributions in practice do not change.By numerical integration and with
E„P ~10
eV (see,e.
g.,Ref. [31)),
we have obtained the best fit to the data (solid line inFig.
1)by meansof
the well-known parame- trization [3]S
'=S, ,
'+Sh; '„,
withS„„=aEP
andS„; h=(242. 6/E)ln(1+1. 2X10 /E+0. 1159E), E
beingmeasured in keV. The fit was performed for the data be- tween
0.
7 and 120keV and we obtainedy„=0.
57 (99de-grees
of
freedom). Other parametrization functions fur- nished bad valuesof g, .
So, our methodology makes it possibleto
argue quantitatively that the present result isa good approximation tothe real stopping power. Figure 3 shows a comparisonof
the best-fitting function (curve b)FIG.
3. Comparison between the proton stopping power in Hz, curve afrom Ref. [3),and the region (the dotted area) ofac- ceptable behaviors for the antiproton one. Curve bisour best- fitting function and curves cand dare examples oflimiting ac- ceptable behaviors. A fast rise below 0.7 keV, necessary to ex- plain the data but not used in the fit, is indicated by a dotted line.with that for the proton (curve a ).
The best-fitting value for S&, did not affect the behav- ior
of S
at high energies.Its
relative importance is,e.
g.,1%
at 10 MeV.Furthermore, an increase
of 5
below0.
7 keV is neces- sary in order to explain the experimental data. This is clearly shown inFig. 4. It
appears that, even by assum-1600—
1400
1200
1000
800
600
400
200
|0
20 30 40 50 60 70 80 Path length (cm)FIG.
4. Comparison between experimental data at 2.1mbar hydrogen pressure and proton behavior after Andersen and Ziegler [3],withE„, ~
10eV,t„, =
200 ns, curve a&,andt„, =0
ns, curve a2.
4520
BRIEF
REPORTSing
t„, =0,
no agreement with the data can be obtained by using an extrapolation down to zero proportional to U,as used for protons by Andersen and Ziegler
[3].
Thisconclusion is independent from the circumstance that in (1)we use R projected, that we measure, instead
of R.
In order to explain the experimental data without a fast riseof S
we would need areduction (and not an increase)of
R by afactor10.
The following remarks may bedrawn.
(i)Between 10 and 120 keV the mean p stopping power in H2 is systematically lower than that
of
proton. We re- call that Sdrensen [9]evaluated p stopping power about half thatof
proton below the stopping maximum.(ii) The maximum in the p stopping power is
=(60+13)% of
that for proton.(iii) The p stopping power crosses that
of
the proton below 10keV.(iv) With such a p stopping-power behavior, the cas- cade times at the three pressures
p„p2,
and p3 turn outto be
100+10, 135+15,
and200+25
ns, in good agree- ment with our previous conclusions[30].
In conclusion, the Barkas effect forhydrogen shows up clearly. We answer positively also asto the existence
of
a maximum in the antiproton stopping power, as for pro- ton, a question that has been posed; see,e.
g.,Refs. [9,16].
Finally a fast rise
of
the stopping power below0.
7keV is observed, in agreement with the qualitative previsions [6,7] originally proposed by Fermi and Teller[10],
and evaluated for hydrogen by Wightman[5].
A riseof
the stopping power near zero kinetic energy was highlighted in thep
stopping cross section evaluation by Cohen[32],
and indicated also by the indirect measurementof
the energy lossof p
in helium by Kottmann[33].
Many thanks are due to Professor
E.
Zavattini for use- ful discussions and suggestions, and to ProfessorG.
Manuzio for valuable discussions during the preparation
of
this manuscript.[1]N.Bohr, Philos. Mag. 25, 10(1913).
[2]H.Bethe, Ann. Phys. (Leipzig) 5, 325(1930).
[3]Hydrogen Stopping Powers and Ranges in Ail Elements, edited by H. H. Andersen and
J. F.
Ziegler (Pergamon, New York, 1977).[4]R.Golser and D.Semrad, Nucl. Instrum. Methods B69, 18(1992).
[5] A.S.Wightman, Phys. Rev. 77,521(1950).
[6] M.Kimura and M.Inokuti, Phys. Rev.A38, 3801 (1988).
[7]D.L.Morgan, Jr.,Hyperfine Interact. 44,399 (1988).
[8]A.M.Ermolaev, Hyperfine Interact. 44, 375(1988).
[9] A. H.Se(rensen, Nucl. Instrum. Methods B48, 10(1990).
[10]
E.
Fermi andE.
Teller, Phys. Rev. 72, 399 (1947).[11]W. H. Barkas,
J.
N. Dyer, and H. H. Heckman, Phys.Rev. Lett. 11,26(1963).
[12]
J.
C.Ashley,R.
H. Ritchie, and W.Brandt, Phys. Rev. B 5, 2392(1972).[13]
J.
Lindhard, Nucl. Instrum. Methods 132,1(1976).[14]G.Basbas, Nucl. Instrum. Methods B4, 227(1984).
[15] C.D.Hu and
E.
Zaremba, Phys. Rev.B37,9268(1988).[16] H. H. Mikkelsen and P.Sigmund, Phys. Rev. A 40, 101 (1989).
[17]S. P.Me(lier, Nucl. Instrum. Methods B 48, 1(1990).
[18] H. H.Mikkelsen, H. Esbensen, and P.Sigmund, Nucl. In- strum. Methods B 48,8(1990).
[19]H. H. Mikkelsen and E.H. Mortensen, Nucl. Instrum.
Methods B48, 39(1990).
[20]D. Semrad, Ch. Eppacher, and
R.
Tober, Nucl. Instrum Methods B48,79(1990).[21] H.Bichsel, Phys. Rev.A41,3642(1990).
[22]
I.
Nagy,B.
Apagyi, andK.
Ladanyi, Phys. Rev. A 42, 1806(1990).[23]
I.
Nagy etal., Phys. Rev.B44, 12 172(1991).[24]
R.
Medenwaldt et al. , Nucl. Instrum. Methods B58, 1(1991).
[25]
R.
Medenwaldt etal.,Phys. Lett. A 155,155(1991).[26]L.H.Andersen etal ,Phys. R.ev.Lett. 62,1731(1989).
[27]L.H.Andersen etal., Phys. Rev.A41, 6536 (1990).
[28]H.Knudsen and
J. F.
Reading, Phys. Rep. 212,107(1992).[29]
R.
Bacher etal., Phys. Rev. A38, 4395 (1988).[30] A.Adamo etal.,Phys. Lett.B285, 15(1992).
[31]
J.
S.Cohen, Phys. Rev.A36,2024(1987).[32]
J.
S.Cohen, Phys. Rev. A 27, 167(1983).[33]